Captain America and Green Lantern

I think that Steve Rogers and Hal Jordan would work very well together.  Hal is known for his will power and Cap arguably has the strongest will of any hero in the Marvel Universe.  The real question is how long Sinestro would put up with being partnered with Arnim Zola!

Cap met the Alan Scott GL in STF #372 and then again in STF #719...

Arnim Zola and The Penguin

If you told me a year ago that these two villains would each make memorable live action appearances I would not have believed it, and yet that has come to pass.  Arnim Zola's unexpected involvement in Captain America: The Winter Soldier was the highlight of the film for me, and that's saying a lot.  Robin Lord Taylor's performance as a young Penguin beginning his criminal empire on Gotham has been entertaining as well, and I look forward to seeing where he winds up by the end of the season.